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Abstract Cities are concentrators of complex, multi‐sectoral interactions. As keystones in the interconnected human‐Earth system, cities have an outsized impact on the Earth system. We describe a multi‐lens framework for organizing our understanding of the complexity of urban systems and scientific research on urban systems, which may be useful for natural system scientists exploring the ways their work can be made more actionable. We then describe four critical dimensions along which improvements are needed to advance the urban research that addresses urgent climate challenges: (a) solutions‐oriented research, (b) equity‐centered assessments which rely on fine‐scale human and ecological data, (c) co‐production of knowledge, and (d) better integration of human and natural systems occurring through theory, observation, and modeling. 

Abstract To demonstrate how a mega city can lead in decarbonizing beyond legal mandates, the city of Los Angeles (LA) developed science-based, feasible pathways towards utilizing 100% renewable energy for its municipally-owned electric utility. Aside from decarbonization, renewable energy adoption can lead to co-benefits such as improving urban air quality from reductions in combustion-related emissions of oxides of nitrogen (NO_x), primary fine particulate matter (PM_2.5) and others. Herein, we quantify changes to air pollutant concentrations and public health from scenarios of 100% renewable electricity adoption in LA in 2045, alongside aggressive electrification of end-use sectors. Our analysis suggests that while ensuring reliable electricity supply, reductions in emissions of air pollutants associated with the 100% renewable electricity scenarios can lead to 8% citywide reductions of PM_2.5concentration while increasing ozone concentration by 5% relative to a 2012 baseline year, given identical meteorology conditions. The combination of these concentration changes could result in net monetized public health benefits (driven by avoided deaths) of up to $1.4 billion in year 2045 in LA, results potentially replicable for other city-scale decarbonization scenarios.